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  • Publication
    Accès libre
    Coherently-averaged dual comb spectrometer at 7.7 µm with master and follower quantum cascade lasers
    (2021-6) ; ;
    Terrasanta, Giulio
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    Gianella, Michele
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    Jouy, Pierre
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    Kapsalidis, Filippos
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    Shahmohammadi Mehran, Mehran
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    Beck Matthias, Matthias
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    Faist, Jérôme
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    Emmenegger, Lukas
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    Hugi, Andreas
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    We demonstrate coherent averaging of the multi-heterodyne beat signal between two quantum cascade laser frequency combs in a master-follower configuration. The two combs are mutually locked by acting on the drive current to control their relative offset frequency and by radio-frequency extraction and injection locking of their intermode beat signal to stabilize their mode spacing difference. By implementing an analog common-noise subtraction scheme, a reduction of the linewidth of all heterodyne beat notes by five orders of magnitude is achieved compared to the free-running lasers. We compare stabilization and post-processing corrections in terms of amplitude noise. While they give similar performances in terms of signal-to-noise ratio, real-time processing of the stabilized signal is less demanding in terms of computational power. Lastly, a proof-of-principle spectroscopic measurement was performed, showing the possibility to reduce the amount of data to be processed by three orders of magnitude, compared to the free-running system.
  • Publication
    Accès libre
    10 kHz linewidth mid-infrared quantum cascade laser by stabilization to an optical delay line
    We present a mid-infrared quantum cascade laser (QCL) with a sub-10 kHz full width at half-maximum linewidth (at 1 s integration time) achieved by stabilization to a free-space optical delay line. The linear range in the center of a fringe detected at the output of an imbalanced Mach–Zehnder interferometer implemented with a short free-space pathlength difference of only 1 m is used as a frequency discriminator to detect the frequency fluctuations of the QCL. Feedback is applied to the QCL current to lock the laser frequency to the delay line. The application of this method in the mid-infrared is reported for the first time, to the best of our knowledge. By implementing it in a simple self-homodyne configuration, we have been able to reduce the frequency noise power spectral density of the QCL by almost 40 dB below 10 kHz Fourier frequency, leading to a linewidth reduction by a factor of almost 60 compared to the free-running laser. The present limits of the setup are assessed and discussed.
  • Publication
    Accès libre
    Electrically-driven pure amplitude and frequency modulation in a quantum cascade laser
    ; ; ;
    Blaser, Stéphane
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    Gresch, Tobias
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    Maulini, Richard
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    Muller, Antoine
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    We present pure amplitude modulation (AM) and frequency modulation (FM) achieved electrically in a quantum cascade laser (QCL) equipped with an integrated resistive heater (IH). The QCL output power scales linearly with the current applied to the active region (AR), but decreases with the IH current, while the emission frequency decreases with both currents. Hence, a simultaneous modulation applied to the current of the AR and IH sections with a proper relative amplitude and phase can suppress the AM, resulting in a pure FM, or vice-versa. The adequate modulation parameters depend on the applied modulation frequency. Therefore, they were first determined from the individual measurements of the AM and FM transfer functions obtained for a modulation applied to the current of the AR or IH section, respectively. By optimizing the parameters of the two modulations, we demonstrate a reduction of the spurious AM or FM by almost two orders of magnitude at characteristic frequencies of 1 and 10 kHz compared to the use of the AR current only.
  • Publication
    Accès libre
    Frequency noise correlation between the offset frequency and the mode spacing in a mid-infrared quantum cascade laser frequency comb
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    Kapsalidis, Filippos
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    Shahmohammadi, Mehran
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    Beck, Mattias
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    Hugi, Andreas
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    Jouy, Pierre
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    Faist, Jérôme
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    The generation of frequency combs in the mid-infrared (MIR) spectral range by quantum cascade lasers (QCLs) has the potential for revolutionizing dual-comb multi-heterodyne spectroscopy in the molecular fingerprint region. However, in contrast to frequency combs based on passively mode-locked ultrafast lasers, their operation relies on a completely different mechanism resulting from a four-wave mixing process occurring in the semiconductor gain medium that locks the modes together. As a result, these lasers do not emit pulses and no direct self-referencing of a QCL comb spectrum has been achieved so far. Here, we present a detailed frequency noise characterization of a MIR QCL frequency comb operating at a wavelength of 8 μm with a mode spacing of ~ 7.4 GHz. Using a beat measurement with a narrow-linewidth single-mode QCL in combination with a dedicated electrical scheme, we measured the frequency noise properties of an optical mode of the QCL comb, and indirectly of its offset frequency for the first time, without detecting it by the standard approach of nonlinear interferometry applied to ultrafast mode-locked lasers. In addition, we also separately measured the noise of the comb mode spacing extracted electrically from the QCL. We observed a strong anti-correlation between the frequency fluctuations of the offset frequency and mode spacing, leading to optical modes with a linewidth slightly below 1 MHz in the free-running QCL comb (at 1-s integration time), which is narrower than the individual contributions of the offset frequency and mode spacing that are at least 2 MHz each.